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Ichimura, Atsushi; Ohyama-Yamaguchi, Tomoko
JSPS-CAS Core University Program seminar. Proceedings of Japan-China joint seminar on atomic and molecular processes in plasma2005
JSPS-CAS Core University Program seminar. Proceedings of Japan-China joint seminar on atomic and molecular processes in plasma2005
AbstractAbstract
[en] A classical field-ionization model is developed for sequential multiple ionization of diatomic and linear triatomic molecules exposed to intense (∼ 1015W/cm2) laser fields. The distance Rion of Coulomb explosion is calculated for a combination of fragment charges, by considering nonadiabatic excitation followed by field ionization associated with the inner and outer saddle points. For diatomic molecules (N2, NO, and I2), the model explains behaviors observed in experiments, as Rion(21→31) < Rion(21→22) between competing charge-asymmetric and symmetric channels, and even-odd fluctuation along a principal pathway. For a triatomic molecule CO2, a comparison of the model with an experiment suggests that charge-symmetric (or nearly symmetric) channels are dominantly populated. (author)
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Koike, Fumihiro (ed.) (Kitasato Univ., Tokyo (Japan)); Chenzhong Dong (ed.) (Northwest Normal Univ., Lanzhou (China)); National Inst. for Fusion Science, Toki, Gifu (Japan); 157 p; Feb 2005; p. 115-120; Japan-China joint seminar on atomic and molecular processes in plasma; Lanzhou (China); 6-11 Mar 2004; 13 refs., 6 figs.
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