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Lange, Steve; Klinkenberg, Martina; Bosbach, Dirk; Deissmann, Guido; Read, David
Proceedings of the second workshop of the HORIZON 2020 CEBAMA project2019
Proceedings of the second workshop of the HORIZON 2020 CEBAMA project2019
AbstractAbstract
[en] The uptake of the long-lived radionuclides Ra and Tc, as well as iodide and molybdate ions by various model phases representative for phases present in hydrated cements was investigated. The model phases were synthesized under argon atmosphere, using well established procedures (e.g., Atkins et al., 1991 and 1992; Baur et al., 2004). Sorption and uptake kinetics by the model phases were studied in static batch experiments under anoxic conditions. Experiments performed for up to 60 days indicate a strong uptake of radium by calcite and CSH phases. Uptake studies performed on iodide revealed the incorporation into AFm-SO. In contrast, no significant uptake of technetium, present as Tc(VII) in solution, by the various model phases was observed. Microanalytical investigations on the uptake of molybdate by AFm phases provided evidence of a molybdate substitution in AFm-SO.
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Altmaier, M.; Montoya, V.; Duro, L.; Valls, A. (eds.); 340 p; ISBN 978-3-7315-0825-0; ; 2019; p. 183-189; 2. Annual Workshop of the Collaborative Project CEBAMA; Espoo (Finland); 16-19 May 2017; ISSN 1869-9669;
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Book
Literature Type
Conference
Country of publication
ALKALINE EARTH ISOTOPES, ALPHA DECAY RADIOISOTOPES, BETA DECAY RADIOISOTOPES, BETA-MINUS DECAY RADIOISOTOPES, BUILDING MATERIALS, CARBON 14 DECAY RADIOISOTOPES, DISPERSIONS, ELEMENTS, EVEN-EVEN NUCLEI, FLUIDS, GASES, HALIDES, HALOGEN COMPOUNDS, HEAVY ION DECAY RADIOISOTOPES, HEAVY NUCLEI, HOMOGENEOUS MIXTURES, HOURS LIVING RADIOISOTOPES, INTERMEDIATE MASS NUCLEI, INTERNAL CONVERSION RADIOISOTOPES, IODINE COMPOUNDS, IODINE ISOTOPES, ISOMERIC TRANSITION ISOTOPES, ISOTOPES, KINETICS, MANAGEMENT, MATERIALS, MIXTURES, MOLYBDENUM COMPOUNDS, NONMETALS, NUCLEI, ODD-EVEN NUCLEI, OXYGEN COMPOUNDS, RADIOACTIVE WASTE MANAGEMENT, RADIOISOTOPES, RADIUM ISOTOPES, RARE GASES, REFRACTORY METAL COMPOUNDS, SOLUTIONS, SOLVATION, TECHNETIUM ISOTOPES, TRANSITION ELEMENT COMPOUNDS, WASTE DISPOSAL, WASTE MANAGEMENT, YEARS LIVING RADIOISOTOPES
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