English, G.A.
Purdue Univ., Lafayette, Ind. (USA)1974
Purdue Univ., Lafayette, Ind. (USA)1974
AbstractAbstract
[en] Cross sections have been determined for 74 nuclides formed in the interaction of natural Ag with 11.5- and 300-GeV protons. The technique of direct gamma-ray spectroscopy was used to determine the yields of nuclides; from this data charge-dispersion and mass-yield curves were constructed for the mass range 7 less than or equal to A less than or equal to 106. The mass-yield curve constructed at 11.5 GeV is seen to agree well with a curve at 29 GeV, the major exception being a plateau in the mass region near the mass of the target. The total reaction cross section obtained by integration of the mass-yield curve at 11.5 GeV is 1.05 +- 0.16b in excellent agreement with a calculated value of 1.13b. A semiempirical calculation predicts a much steeper decrease in the mass-yield than is observed experimentally. The experimental charge dispersions are essentially Gaussian. The full-widths at half-maximum and the difference between the most stable and the most probable charges can be correlated roughly with the transition between a spallation and a two-body breakup mechanism. A semiempirical calculation of charge dispersion predicts higher peak maxima than observed experimentally. (auth)
Original Title
Cross sections for production of 74 nuclides
Primary Subject
Source
1974; 276 p; University Microfilms Order No. 75-17,188.; Thesis (Ph. D.).
Record Type
Report
Literature Type
Thesis/Dissertation
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Firestone, Richard B; Perry, D.L.; English, G.A.; Firestone, R.B.; Leung, K.-N.; Garabedian, G.; Molnar, G.L.; Revay, Zs.
Ernest Orlando Lawrence Berkeley National Laboratory, Berkeley, CA (United States). Funding organisation: Accelerator and Fusion Research Division, Earth Sciences Division, Environment, Health and Safety Division, Nuclear Science Division (United States)2008
Ernest Orlando Lawrence Berkeley National Laboratory, Berkeley, CA (United States). Funding organisation: Accelerator and Fusion Research Division, Earth Sciences Division, Environment, Health and Safety Division, Nuclear Science Division (United States)2008
AbstractAbstract
[en] Prompt gamma activation analysis (PGAA) has been used to analyze metal ion oxyanion materials that have multiple applications, including medicine, materials, catalysts, and electronics. The significance for the need for accurate, highly sensitive analyses for the materials is discussed in the context of quality control of end products containing the parent element in each material. Applications of the analytical data for input to models and theoretical calculations related to the electronic and other properties of the materials are discussed
Primary Subject
Secondary Subject
Source
LBNL--739E; AC02-05CH11231; Available from OSTI as DE00935410; PURL: https://www.osti.gov/servlets/purl/935410-sqHyHA/; Journal Publication Date: April 2008
Record Type
Journal Article
Journal
Journal of Radioanalytical and Nuclear Chemistry; ISSN 0236-5731; ; v. 276(1); p. 13
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Firestone, Richard B; English, G.A.; Firestone, R.B.; Perry, D.L.; Reijonen, J.P.; Leung, Ka-Ngo; Garabedian, G.F.; Molnar, G.L.; Revay, Zs.
Ernest Orlando Lawrence Berkeley National Laboratory, Berkeley, CA (United States). Funding organisation: Accelerator and Fusion Research Division (United States); Earth Sciences Division (United States); Environmental Energy Technologies Division (United States); Nuclear Science Division (United States)2008
Ernest Orlando Lawrence Berkeley National Laboratory, Berkeley, CA (United States). Funding organisation: Accelerator and Fusion Research Division (United States); Earth Sciences Division (United States); Environmental Energy Technologies Division (United States); Nuclear Science Division (United States)2008
AbstractAbstract
[en] Without quality historical records that provide the composition of legacy materials, the elemental and/or chemical characterization of such materials requires a manual analytical strategy that may expose the analyst to unknown toxicological hazards. In addition, much of the existing legacy inventory also incorporates radioactivity, and, although radiological composition may be determined by various nuclear-analytical methods, most importantly, gamma-spectroscopy, current methods of chemical characterization still require direct sample manipulation, thereby presenting special problems with broad implications for both the analyst and the environment. Alternately, prompt gamma activation analysis (PGAA) provides a 'single-shot' in-situ, non-destructive method that provides a complete assay of all major entrained elemental constituents.1-3. Additionally, neutron activation analysis (NAA) using short-lived activation products complements PGAA and is especially useful when NAA activation surpasses the PGAA in elemental sensitivity
Primary Subject
Secondary Subject
Source
LBNL--628E; AC02-05CH11231; Available from OSTI as DE00934995; PURL: https://www.osti.gov/servlets/purl/934995-cHckgD/; Journal Publication Date: July 2008
Record Type
Journal Article
Journal
Journal of Radioanalytical and Nuclear Chemistry; ISSN 0236-5731; ; v. 277(1); p. 5
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AbstractAbstract
[en] Prompt gamma activation analysis (PGAA) has been used to detect and quantify impurities in the analyses of rare earth (RE) oxides. The analytical results are discussed with respect to the importance of having a thorough identification and contaminant elements in these compounds regarding the function of the materials in their various applications. Also, the importance of using PGAA to analyze materials in support of other physico-chemical studies of the materials is discussed, including the study of extremely low concentrations of ions - such as the rare earth ions themselves - in bulk material matrices. (author)
Primary Subject
Source
24 refs.
Record Type
Journal Article
Journal
Journal of Radioanalytical and Nuclear Chemistry; ISSN 0236-5731; ; CODEN JRNCDM; v. 265(2); p. 229-233
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INIS VolumeINIS Volume
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AbstractAbstract
[en] Without quality historical records that provide the composition of legacy materials, the elemental and/or chemical characterization of such materials requires a manual analytical strategy that may expose the analyst to unknown toxicological hazards. In addition, much of the existing legacy inventory also incorporates radioactivity, and, although radiological composition may be determined by various nuclear-analytical methods, most importantly, gamma-spectroscopy, current methods of chemical characterization still require direct sample manipulation, thereby presenting special problems with broad implications for both the analyst and the environment. Alternately, prompt gamma activation analysis (PGAA) provides a 'single-shot' in-situ, non-destructive method that provides a complete assay of all major entrained elemental constituents. Additionally, neutron activation analysis (NAA) using short-lived activation products complements PGAA and is especially useful when NAA activation surpasses the PGAA in elemental sensitivity. (author)
Primary Subject
Source
6 refs.
Record Type
Journal Article
Journal
Journal of Radioanalytical and Nuclear Chemistry; ISSN 0236-5731; ; CODEN JRNCDM; v. 277(1); p. 25-29
Country of publication
Reference NumberReference Number
INIS VolumeINIS Volume
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AbstractAbstract
[en] Prompt gamma activation analysis (PGAA) has been used to analyze metal ion oxyanion materials that have multiple applications, including medicine, materials, catalysts, and electronics. The significance for the need for accurate, highly sensitive analyses for the materials is discussed in the context of quality control of end products containing the parent element in each material. Applications of the analytical data for input to models and theoretical calculations related to the electronic and other properties of the materials are discussed. (author)
Primary Subject
Source
21 refs.
Record Type
Journal Article
Journal
Journal of Radioanalytical and Nuclear Chemistry; ISSN 0236-5731; ; CODEN JRNCDM; v. 276(1); p. 273-277
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AbstractAbstract
[en] Thermal neutrons from the Budapest Research Reactor and fast neutrons from the Berkeley Neutron Generator Facility have been used to analyze uranium. It has been shown that both prompt and delayed gamma-rays from neutron capture and fission product decay can be used to analyze uranium concentrations and 235U enrichment. Detection of neutrons from the spontaneous fission of 238U has been demonstrated for uranium analysis. The observation of high-energy gamma-rays following the decay of short-lived fission products is a sensitive indication of fissile material, and the ratio of fission product gamma-ray intensities can uniquely determine the concentrations of fission isotopes. (author)
Primary Subject
Secondary Subject
Source
14efs.
Record Type
Journal Article
Journal
Journal of Radioanalytical and Nuclear Chemistry; ISSN 0236-5731; ; CODEN JRNCDM; v. 265(2); p. 241-245
Country of publication
ACTINIDE NUCLEI, ACTINIDES, ALPHA DECAY RADIOISOTOPES, BARYON REACTIONS, DECAY, ELECTROMAGNETIC RADIATION, ELEMENTS, EVEN-EVEN NUCLEI, EVEN-ODD NUCLEI, FISSION, FISSIONABLE MATERIALS, HADRON REACTIONS, HEAVY NUCLEI, INTERNAL CONVERSION RADIOISOTOPES, IONIZING RADIATIONS, ISOMERIC TRANSITION ISOTOPES, ISOTOPES, MATERIALS, METALS, MINUTES LIVING RADIOISOTOPES, NEUTRON REACTIONS, NUCLEAR DECAY, NUCLEAR REACTIONS, NUCLEI, NUCLEON REACTIONS, RADIATIONS, RADIOACTIVE MATERIALS, RADIOISOTOPES, SEPARATION PROCESSES, SPONTANEOUS FISSION RADIOISOTOPES, URANIUM ISOTOPES, YEARS LIVING RADIOISOTOPES
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