[en] Beijing aerosols are characterised for the 2003-2004 period using an inclusive experimental set up for aerosol mass, chemistry and number, deployed at three sites. Aerosol size segregation in two fractions (fine and coarse) appears appropriated for source identification and investigations about gas-to-particle interactions. Several various sources contribute to air pollution: traffic, coal burning and industrial activities. The present study also shows how summer aerosol is influenced by the photochemical formation of secondary particles, and the significant amount of coarse and fine mineral dust all year long. Coal burning in winter has a lower influence than assessed in the past. The origin and altitude of the air masses entering Beijing are of key interest to understand the ageing of pollutants and their regional redistribution. By its expected effects onto these regional parameters, climate change may strongly affect Beijing air pollution in the coming decades. (author)

[en] This paper summarizes the creation and technical evolution of atomic time scales, recalling the parallel development of their acceptance and the remaining problems. We consider a consequence of the accuracy of time measurement, i.e. the entry of Einstein's general relativity into metrology and its applications. We give some details about the method of calculation and the characteristics of International Atomic Time, and we show how it is disseminated at the ultimate level of precision. (authors)

[en] Beijing aerosols are scrutinized as a case study for atmospheric interactions in a complex multi-source situation. For the first time, fine (≤ 2 μm) and coarse (≥ 2 μm) aerosols were continuously collected during a time period (20 months) long enough to capture seasonal trends of sources and interactions. Weekly samples were obtained from January 2003 to August 2004 downtown and during 9 months at two peri-urban sites. Aerosol samples were chemically characterized (black carbon (BC), organic carbon (OC), and major ions) and dust was obtained from mass closure. Concentration data were smoothed and boundary layer height (BLH) corrected in order to better identify sources and processes. All yearlong, the coarse aerosol is dominated by dust (75%) whereas the fine mode is dominated (46%) by carbonaceous particles. Photochemistry is an intense driving force for secondary aerosol formation including secondary organic aerosol (SOA). Dust particles present a reactive surface for secondary aerosol formation from the intense anthropogenic pool of acidic gaseous precursors (SO₂, HNO₃, and volatile organic compounds (VOCs)). These interactions favor the formation of a very significant coarse fraction for SO₄, NO₃, and POM, a feature almost never encountered in developed countries. Surprisingly too is the presence of fine NH₄NO₃ in summer. A new result is also that the winter 'heating season' appears at present of minor importance with, however, a significant component from domestic heating as traced by BC/OC. In the future, traffic is likely to dominate downtown anthropogenic emissions. Year-to-year variability in meteorological conditions is likely to influence inputs from arid regions and from regional industrial and biomass burning sources. (authors)

[en] The Mediterranean basin is one of the most sensitive regions in the world regarding climate change and air quality. Deserts and marine aerosols combine with combustion aerosols from maritime traffic, large urban centers, and at a larger scale from populated industrialized regions in Europe. From Tetouan city located in the North of Morocco, we attempted to better figure out the main aerosol transport pathways and their respective aerosol load and chemical profile by examining air mass back trajectory patterns and aerosol chemical compositions from May 2011 to April 2012. The back trajectory analysis throughout the sampling period led to four clusters, for which meteorological conditions and aerosol chemical characteristics have been investigated. The most frequent cluster (CL3: 39%) corresponds to polluted air masses coming from the Mediterranean Basin, characterized by urban and marine vessels emissions out of Spain and of Northern Africa. Two other polluted clusters were characterized. One is of local origin (CL1: 22%), with a marked contribution from urban aerosols (Rabat, Casablanca) and from biomass burning aerosols. The second (CL2: 32%) defines air masses from the near Atlantic Ocean, affected by pollutants emitted from the Iberian coast. A fourth cluster (CL4: 7%) is characterized by rather clean, fast and rainy oceanic air masses, influenced during their last 24 h before reaching Tetouan by similar sources with those affecting CL2, but to a lesser extent. The chemical data show that carbonaceous species are found in the fine aerosols fraction and are generally from local primary sources (low OC/EC) rather than long-range transported. In addition to fresh traffic and maritime vessel aerosols, our results suggest the contribution of local biomass burning. (author)

[en] The aim of our program is to determine past, present and future emission inventories of carbonaceous particles from 1860 to 2100 for fossil fuel and biofuel sources. Emission inventories for savannah and forest fires have been developed by using burnt area products given by satellite for Asia and Africa. The strong collaboration with the different groups attending this GICC program has allowed to develop the following results. 1- With the improvement of algorithms and new choices for emission factors, emission inventories for black carbon (BC), primary organic carbon (OCp) and total organic carbon (OCtot) have been constructed for the period 1950 to 1997 for fossil fuel and biofuel sources. With these new development, biofuel sources have been seen to be significant, especially in the developing countries. 2- Past inventories have been developed for fossil fuel and biofuel sources from 1860 to 1997 by taking into account the evolution of fuel consumption, fuel use and emission factors. 3- Savannah and forest fire inventories have been constructed based on burnt area products, for Africa (1981-1991, 2000) and Asia (2000-2001). These results show the importance of using real time data instead of statistics. 4-Future emission inventory of black carbon by fossil fuel sources has been constructed for 2100 following the IPCC scenario A2 (catastrophic case) and B1 (perfect world). 5-Characterization of biofuel emissions has been realized by organizing an experiment in a combustion chamber where indian and chinese biofuels (fuelwood, agricultural wastes, dung-cake etc..). were burnt, reproducing the burning methods used in these countries. 6-Finally, the differences between the existing inventories of carbonaceous aerosols has been explained. (A.L.B.)

[en] Global environmental and climate conditions fluctuate on all kind of spatio-temporal scales. Some fluctuations or change/trends are not only anthropogenic, but have different regional and national signatures. While the frequency of extreme events on smaller scales is changing, the public sector and general opinion become more and more aware and concerned of local impacts from global environmental and climate changes. Indeed, negative effects and feedbacks, might occur on ecosystems, natural resources, buildings and grounds, superstructures, economies, food security, public health. This is how, during 1999, a concerted French initiative led to the research program 'Management and Impacts of Climate Change' (GICC). GICC is essentially managed by the Ministry of Ecology and Sustainable Development in close collaboration with the Inter-Ministerial Mission on Greenhouse Effect (MIES). GICC started in 1999. Its first phase (1999-2006) included four calls for proposal (1999, 2000, 2001, and 2002). In parallel and in 2003-2004, the MIES has been developing the so-called 'Climate Plan' based upon three principles : Insure that France follows agreements from the 'Kyoto Protocol'; Participate in ways and means leading to reduction of greenhouse gases by 75% in 2050; Allow for reduction of pollution from transportation means. Input from GICC Phase One final reports are contributing to 'Climate Plan'. The eight themes proposed by GICC-1 (1999-2002) are as follows: Theme 1: Evolution scenarios of the average and extreme features of the 21. Century climate; Theme 2: Interactions between climate, economy and society; related timescales; Theme 3: Role of carbon forest uptake and agricultural practices on climate policies; Theme 4: Links between national and international activities; Theme 5: Towards new inventories of GHG and aerosols (direct and indirect) emissions; Theme 6: Impacts on terrestrial biosphere; Theme 7: Impacts on hydro-systems; Theme 8: Impacts on public health. A symposium presenting the available results of the GICC first phase has taken place in MEDD, Paris, November 23-24, 2004. A final presentation workshop of the first phase took place in Paris, on May 11-12, 2006. This document is the proceedings of this scientific restitution seminar. It is organized in 9 sessions which follow the 8 themes listed above plus a round table for the status and perspectives of the GICC program. (J.S.)