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Menlove, H.O.; Eccleston, G.W.
Los Alamos National Lab., NM (United States). Funding organisation: USDOE, Washington, DC (United States)1992
Los Alamos National Lab., NM (United States). Funding organisation: USDOE, Washington, DC (United States)1992
AbstractAbstract
[en] In recent years, both passive- and active-neutron nondestructive assay (NDA) systems have been used to measure the uranium and plutonium content in 200-ell drums. Because of the heterogeneity of the wastes, representative sampling is not possible and NDA methods are preferred over destructive analysis. Active-neutron assay systems are used to measure the fissile isotopes such as 235U, 23Pu, and 241Pu; the isotopic ratios are used to infer the total plutonium content and thus the specific disintegration rate. The active systems include 14-MeV-neutron (DT) generators with delayed-neutron counting, (D,T) generators with the differential die-away technique, and 252Cf delayed-neutron shufflers. Passive assay systems (for example, segmented gamma-ray scanners)5 have used gamma-ray sessions, while others (for example, passive drum counters) used passive-neutron signals. We have developed a new passive-neutron measurement technique to improve the accuracy and sensitivity of the NDA of plutonium scrap and waste. This new 200-ell-drum assay system combines the classical NDA method of counting passive-neutron totals and coincidences from plutonium with the new features of ''add-a-source'' (AS) and multiplicity counting to improve the accuracy of matrix corrections and statistical techniques that improve the low-level detectability limits. This paper describes the improvements we have made in passive-neutron assay systems and compares the accuracies and detectability limits of passive- and active-neutron assay systems
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1992; 21 p; Transuranic waste characterization conference; Pocatello, ID (United States); 10-12 Aug 1992; CONF-920882--2; CONTRACT W-7405-ENG-36; OSTI as DE92040385; NTIS; INIS; US Govt. Printing Office Dep
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Report
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Conference
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ACTINIDE NUCLEI, ACTINIDES, ALPHA DECAY RADIOISOTOPES, CALIFORNIUM ISOTOPES, CHEMICAL ANALYSIS, ELEMENTS, EVEN-EVEN NUCLEI, HEAVY NUCLEI, ISOTOPES, MANAGEMENT, MATERIALS, METALS, NUCLEI, RADIOACTIVE MATERIALS, RADIOACTIVE WASTES, RADIOISOTOPES, TRANSURANIUM ELEMENTS, WASTES, YEARS LIVING RADIOISOTOPES
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