[en] Site-specific radiological performance assessments are required for the disposal of low-level radioactive waste (LLW) at both commercial and US Department of Energy facilities. This work explores source term modeling of LLW disposal facilities by using two state-of-the-art computer codes, SOURCEI and SOURCE2. An overview of the performance assessment methodology is presented, and the basic processes modeled in the SOURCE1 and SOURCE2 codes are described. Comparisons are made between the two advective models for a variety of radionuclides, transport parameters, and waste-disposal technologies. These comparisons show that, in general, the zero-order model predicts undecayed cumulative fractions leached that are slightly greater than or equal to those of the first-order model. For long-lived radionuclides, results from the two models eventually reach the same value. By contrast, for short-lived radionuclides, the zero-order model predicts a slightly higher undecayed cumulative fraction leached than does the first-order model. A new methodology, based on sensitivity and uncertainty analyses, is developed for predicting intruder scenarios. This method is demonstrated for ¹³⁷Cs in a tumulus-type disposal facility. The sensitivity and uncertainty analyses incorporate input-parameter uncertainty into the evaluation of a potential time of intrusion and the remaining radionuclide inventory. Finally, conclusions from this study are presented, and recommendations for continuing work are made