Development of a process for the separation of MA(III) from Ln(III) fission products using HONTA impregnated adsorbent
AbstractAbstract
[en] To minimize the use of organic solvents and achieve a selective adsorption separation of minor actinides (MA(III)) and Ln(III), adsorbents consisting of SiO2-P particles impregnated with hexaoctylnitrilotriacetamide (HONTA) were prepared. Batch experiments were performed to evaluate the adsorption properties of the HONTA/SiO2-P adsorbent for MA(III) and simulated fission products in HNO3 solution. The uniform distribution of Eu(III) on the adsorbent was confirmed via particle-induced X-ray emission analysis, and X-ray photoelectron spectroscopy revealed that EuNO3 was the adsorbed species. This study provides a simplified process for the separation of MA(III) using a HONTA/SiO2-P-packed column. (author)
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Journal Article
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Journal of Radioanalytical and Nuclear Chemistry; ISSN 0236-5731; ; CODEN JRNCDM; v. 333(5); p. 2413-2420
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