AbstractAbstract
[en] Spontaneous fission and α-decay of 253-257104 and 258106 were investigated in irradiations of 204,206,208Pb with 50Ti and 209Bi with 51V, respectively. New spontaneous fission activities were identified and assigned to 253104, 254104, and 258106. The half-lives were measured as T1/2=(48+17-10) μs for 253104, T1/2=(23±3) μs for 254104, and T1/2=(2.9+1.3-0.7) ms for 258106. No indication for α-decay of any of these isotopes was found. For the α-decay branching ratios bα limits corresponding to bα≤0.1 for 253104, bα≤0.015 for 254104, and bα≤0.2 for 258106 were obtained. These results prove a reduced fission probability for nuclei with neutron numbers N=152 up to Z=106 and a steep decrease of the fission half-lives for neutron numbers N < 152 up to element 104. α-decay data of 257104 and 255104 have been improved. An isomeric state decaying by α-emission was identified in 257104 and attributed to a low lying 11/2-[725] state. A small α-decay branch for the even-even nucleus 256104, indicated in an earlier experiment at SHIP, was confirmed, allowing a better founded extrapolation of experimental masses for even-even nuclei up to 264Hs (Z=108), the heaviest even-even nucleus identified so far. (orig.)
Primary Subject
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Source
With 10 figs., 5 tabs., 37 refs.
Record Type
Journal Article
Literature Type
Numerical Data
Journal
Zeitschrift fuer Physik. A, Hadrons and Nuclei; ISSN 0939-7922; ; CODEN ZPAHEX; v. 359(4); p. 415-425
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AbstractAbstract
[en] Isotopes of dubnium (element 105) with mass numbers A = 256, 257, and 258 were produced by the reaction 209Bi(50Ti,xn) 259-xDb (x = 1, 2, 3) at projectile energies of (4.59-5.08) AMeV. Excitation functions were measured for the 1n, 2n and 3n evaporation channels. The same position of the excitation function was observed for the 1n channel as for the previously measured 1n channel of the reaction 208Pb(50Ti,1n)257Rf. The measured α-decay data of 257Db and its daughter products resulted in the identification of α-decaying isomeric states in 257Db and 253Lr. Two new isotopes, 256Db and 252Lr, were produced at the highest bombarding energies of 4.97 AMeV and 5.08 AMeV. They were identified by delayed α-α coincidences. The measured half-lives are (1.6+0.5-0.3) s for 256Db and (0.36+0.11-0.07) s for 252Lr. Besides α-decay, a spontaneous fission activity of T1/2 = (2.3+1.1-0.6) s was observed and attributed to an electron-capture branch of 256Db, which feeds the fissioning nucleus 256Rf. A branching ratio of 0.36±0.12 was obtained. The isotope 255Rf was produced by the reaction 207Pb(50Ti,2n)255Rf. Improved decay data have been obtained by means of α- and α-γ spectroscopy. (orig.)
Primary Subject
Record Type
Journal Article
Literature Type
Numerical Data
Journal
European Physical Journal. A; ISSN 1434-6001; ; v. 12(1); p. 57-67
Country of publication
ALPHA DECAY, ALPHA SPECTRA, BISMUTH 209 TARGET, BRANCHING RATIO, ELEMENT 104 255, ELEMENT 105 256, ELEMENT 105 257, ENERGY SPECTRA, EXCITATION FUNCTIONS, EXPERIMENTAL DATA, HALF-LIFE, HEAVY ION FUSION REACTIONS, INTEGRAL CROSS SECTIONS, ISOMERIC NUCLEI, LAWRENCIUM 252, LAWRENCIUM 253, LEAD 207 TARGET, MEV RANGE 100-1000, NEUTRONS, SPONTANEOUS FISSION, TITANIUM 50 REACTIONS
ACTINIDE NUCLEI, ALPHA DECAY RADIOISOTOPES, BARYONS, CROSS SECTIONS, DATA, DECAY, ELEMENT 104 ISOTOPES, ELEMENT 105 ISOTOPES, ELEMENTARY PARTICLES, ENERGY RANGE, EVEN-ODD NUCLEI, FERMIONS, FISSION, FUNCTIONS, HADRONS, HEAVY ION REACTIONS, HEAVY NUCLEI, INFORMATION, ISOTOPES, LAWRENCIUM ISOTOPES, MEV RANGE, NUCLEAR DECAY, NUCLEAR REACTIONS, NUCLEI, NUCLEONS, NUCLEOSYNTHESIS, NUMERICAL DATA, ODD-EVEN NUCLEI, ODD-ODD NUCLEI, RADIOISOTOPES, SECONDS LIVING RADIOISOTOPES, SPECTRA, SPONTANEOUS FISSION RADIOISOTOPES, SYNTHESIS, TARGETS
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INIS IssueINIS Issue
AbstractAbstract
No abstract available
Original Title
Zerfallseigenschaften neutronenarmer Isotope der Elemente Z=103-106
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Source
1999 spring meeting of Fachverband Physik der Hadronen und Kerne of Deutsche Physikalische Gesellschaft e.V. (DPG), with physics and book exhibition; Fruehjahrstagung 1999 des Fachverbandes Physik der Hadronen und Kerne der Deutschen Physikalischen Gesellschaft e.V. (DPG) - mit Physik- und Buchausstellung; Freiburg im Breisgau (Germany); 22-26 Mar 1999
Record Type
Journal Article
Literature Type
Conference; Numerical Data
Journal
Verhandlungen der Deutschen Physikalischen Gesellschaft; ISSN 0420-0195; ; CODEN VDPEAZ; v. 34(3); p. 101
Country of publication
ALPHA DECAY, DE-EXCITATION, DELAYED GAMMA RADIATION, ELEMENT 104 253, ELEMENT 104 254, ELEMENT 104 255, ELEMENT 104 257, ELEMENT 105 257, ELEMENT 105 COMPOUNDS, ELEMENT 106 ISOTOPES, ENERGY SPECTRA, EXPERIMENTAL DATA, GAMMA SPECTRA, HALF-LIFE, HIGH SPIN STATES, LAWRENCIUM 253, MICROSEC LIVING RADIOISOTOPES, MILLISEC LIVING RADIOISOTOPES, NOBELIUM 251, ROTATIONAL STATES, SPONTANEOUS FISSION
ACTINIDE NUCLEI, ALPHA DECAY RADIOISOTOPES, DATA, DECAY, ELECTROMAGNETIC RADIATION, ELEMENT 104 ISOTOPES, ELEMENT 105 ISOTOPES, ENERGY LEVELS, ENERGY-LEVEL TRANSITIONS, EVEN-EVEN NUCLEI, EVEN-ODD NUCLEI, EXCITED STATES, FISSION, GAMMA RADIATION, HEAVY NUCLEI, INFORMATION, IONIZING RADIATIONS, ISOTOPES, LAWRENCIUM ISOTOPES, NOBELIUM ISOTOPES, NUCLEAR DECAY, NUCLEAR REACTIONS, NUCLEI, NUMERICAL DATA, ODD-EVEN NUCLEI, RADIATIONS, RADIOISOTOPES, SECONDS LIVING RADIOISOTOPES, SPECTRA, SPONTANEOUS FISSION RADIOISOTOPES, TRANS 104 ELEMENT COMPOUNDS, TRANSPLUTONIUM COMPOUNDS, TRANSURANIUM COMPOUNDS
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AbstractAbstract
[en] The progress in investigations of the heaviest known elements in the recent years was only possible with an elaborate target technology. Large area thin and homogeneous targets of Pb and Bi, mounted on a rotating wheel to allow high projectile currents, were used in the experiments performed at the velocity filter SHIP at GSI Darmstadt. Various techniques for the on-line monitoring of the targets will be described and their importance for the experiments will be discussed. The experimental results from the investigations of the heaviest elements will be summarized briefly. (orig.)
Primary Subject
Secondary Subject
Source
14. world conference of the International Nuclear Target Development Society (INTDS): Heavy-ion targets and related phenomena; Darmstadt (Germany, F.R.); 5-9 Sep 1988
Record Type
Journal Article
Literature Type
Conference; Numerical Data
Journal
Nuclear Instruments and Methods in Physics Research, Section A; ISSN 0168-9002; ; CODEN NIMAE; v. 282(1); p. 28-35
Country of publication
BEAM MONITORING, BEAM POSITION, BISMUTH 209 TARGET, ELEMENT 104 255, ELEMENT 104 256, ELEMENT 104 257, ENERGY DEPENDENCE, ENERGY LOSSES, EXCITATION FUNCTIONS, EXPERIMENTAL DATA, HEAVY ION FUSION REACTIONS, INTEGRAL CROSS SECTIONS, LEAD 208 TARGET, MEV RANGE 100-1000, MILLISEC LIVING RADIOISOTOPES, NEUTRONS, ON-LINE CONTROL SYSTEMS, ROTATION, RUTHERFORD SCATTERING, SPONTANEOUS FISSION RADIOISOTO, TARGET CHAMBERS, TITANIUM 50 REACTIONS, X-RAY DETECTION
ACCELERATOR FACILITIES, ALPHA DECAY RADIOISOTOPES, BARYONS, CONTROL SYSTEMS, CROSS SECTIONS, DATA, DETECTION, ELASTIC SCATTERING, ELEMENT 104 ISOTOPES, ELEMENTARY PARTICLES, ENERGY RANGE, EVEN-EVEN NUCLEI, EVEN-ODD NUCLEI, FERMIONS, HADRONS, HEAVY ION REACTIONS, INFORMATION, ISOTOPES, MEV RANGE, MONITORING, NUCLEAR REACTIONS, NUCLEI, NUCLEONS, NUCLEOSYNTHESIS, NUMERICAL DATA, ON-LINE SYSTEMS, RADIATION DETECTION, RADIOISOTOPES, SCATTERING, SECONDS LIVING RADIOISOTOPES, SYNTHESIS, TARGETS
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AbstractAbstract
[en] Measured α-decay spectra of the isotopes 215Th and 213Ra were used to investigate the influence of energy summing of α-particles and conversion electrons, and Auger electrons, respectively, emitted after α-decays into excited daughter levels, on the shape of α-spectra. The isotopes were produced in heavy ion fusion reactions and were implanted into silicon surface barrier detectors after in-flight separation from the projectile beam. It was shown that the summing effects will cause (a) the occurrence of additional lines in the α-energy spectra and (b) a change in the relative intensities of α-lines belonging to the α-decay pattern of a certain isotope. The results for 215Th and 213Ra are used for a discussion of the α-decay properties of the isotope 255104 and its α-decay products 251No and 247Fm. Especially the large discrepancies of the α-energies of 247Fm measured in our experiments and literature values are interpreted as due to a summing between α and electron energies. (orig.)
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Secondary Subject
Record Type
Journal Article
Literature Type
Numerical Data
Journal
Nuclear Instruments and Methods in Physics Research, Section A; ISSN 0168-9002; ; CODEN NIMAE; v. 274(3); p. 522-527
Country of publication
ALPHA DECAY, ALPHA SPECTRA, AUGER EFFECT, CALCIUM 48 REACTIONS, ELECTRON SPECTRA, ELEMENT 104 255, ENERGY SPECTRA, ERBIUM 170 TARGET, EXPERIMENTAL DATA, GAMMA SPECTRA, HEAVY ION FUSION REACTIONS, INTERNAL CONVERSION RADIOISOTO, K CONVERSION, LEVEL WIDTHS, MEV RANGE 100-1000, MILLISEC LIVING RADIOISOTOPES, NEUTRONS, RADIUM 213, SPONTANEOUS FISSION RADIOISOTO, THORIUM 215, TITANIUM 50 REACTIONS, X-RAY SPECTRA, YTTERBIUM 172 TARGET
ACTINIDE NUCLEI, ALPHA DECAY RADIOISOTOPES, BARYONS, BETA DECAY RADIOISOTOPES, CONVERSION, DATA, DECAY, ELECTRON CAPTURE RADIOISOTOPES, ELEMENT 104 ISOTOPES, ELEMENTARY PARTICLES, ENERGY RANGE, EVEN-ODD NUCLEI, FERMIONS, HADRONS, HEAVY ION REACTIONS, HEAVY NUCLEI, INFORMATION, INTERNAL CONVERSION, ISOMERIC TRANSITION ISOTOPES, ISOTOPES, MEV RANGE, MINUTES LIVING RADIOISOTOPES, NUCLEAR DECAY, NUCLEAR REACTIONS, NUCLEI, NUCLEONS, NUCLEOSYNTHESIS, NUMERICAL DATA, RADIOISOTOPES, RADIUM ISOTOPES, SECONDS LIVING RADIOISOTOPES, SPECTRA, SYNTHESIS, TARGETS, THORIUM ISOTOPES
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AbstractAbstract
[en] Evaporation residues from the fusion reactions 48Ca+206,208Pb and 50Ti+207,208Pb, 209Bi were investigated using the velocity filter SHIP. Four new isotopes 258,257105 and 254,253Lr were identified and α decay of 255104 and 256104 was observed for the first time. A hindrance to complete fusion by a factor of about 30 at bombarding energies close to the classical barrier was deduced from a measured excitation function for 50Ti+208Pb. The mass extents for 256104 and 260106, obtained from their α-decay energies, were used to determine the ground-state shell effects and a semi-empirical description of the half-life TSF for even-even nuclei. The abrupt decrease in TSF for elements from nobelium to element 104 was found to be correlated with a decrease in the fission barrier width, which we regard as confirmation of the expected drop in the outer fission barrier to below the ground state. The total kinetic energies released in SF of 256104 and 258104 were measured and found to be 207±13 MeV and 220±15 MeV respectively. These values agree with those predicted from empirical systematics. (orig.)
Primary Subject
Source
International conference on actinides (Actinides '85); Aix-en-Provence (France); 2-6 Sep 1985
Record Type
Journal Article
Literature Type
Conference; Numerical Data
Journal
Country of publication
ALPHA DECAY, BISMUTH 209 TARGET, CALCIUM 48 REACTIONS, ELEMENT 104 255, ELEMENT 104 256, ELEMENT 105 257, ELEMENT 105 258, EXCITATION FUNCTIONS, EXPERIMENTAL DATA, FISSION BARRIER, HALF-LIFE, HEAVY ION FUSION REACTIONS, KINETIC ENERGY, LAWRENCIUM 253, LAWRENCIUM 254, LEAD 206 TARGET, LEAD 207 TARGET, LEAD 208 TARGET, MILLISEC LIVING RADIOISOTOPES, NEUTRON-DEFICIENT ISOTOPES, SPONTANEOUS FISSION, SPONTANEOUS FISSION RADIOISOTO, TITANIUM 50 REACTIONS
ACTINIDE NUCLEI, ALPHA DECAY RADIOISOTOPES, BETA DECAY RADIOISOTOPES, DATA, DECAY, ELECTRON CAPTURE RADIOISOTOPES, ELEMENT 104 ISOTOPES, ELEMENT 105 ISOTOPES, ENERGY, EVEN-EVEN NUCLEI, EVEN-ODD NUCLEI, FISSION, HEAVY ION REACTIONS, HEAVY NUCLEI, INFORMATION, ISOTOPES, LAWRENCIUM ISOTOPES, NUCLEAR DECAY, NUCLEAR REACTIONS, NUCLEI, NUCLEOSYNTHESIS, NUMERICAL DATA, ODD-EVEN NUCLEI, ODD-ODD NUCLEI, POTENTIAL ENERGY, RADIOISOTOPES, SECONDS LIVING RADIOISOTOPES, SYNTHESIS, TARGETS
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AbstractAbstract
[en] The author reviews the experiments for the production of the elements 104-109, performed at the GSI Darmstadt using the UNILAC and the SHIP spectrometer. Furthermore shell effects in collision dynamics are discussed. (HSI)
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Source
Kienle, P.; Ricci, R.A.; Rubbino, A. (eds.); Societa Italiana di Fisica, Bologna (Italy); 623 p; ISBN 0-444-87114-4; ; 1989; p. 282-320; North-Holland; Amsterdam (Netherlands); International School of Physics 'Enrico Fermi'. 103. course: Trends in nuclear physics; Varenna (Italy); 23 Jun - 3 Jul 1987
Record Type
Book
Literature Type
Conference; Progress Report
Country of publication
ALPHA DECAY, BISMUTH 209 TARGET, CHROMIUM 54 REACTIONS, ELEMENT 104 255, ELEMENT 104 256, ELEMENT 104 258, ELEMENT 105 257, ELEMENT 106 260, ELEMENT 107 261, ELEMENT 107 262, ELEMENT 108 264, ELEMENT 108 265, ELEMENT 109 266, EVAPORATION MODEL, FISSION BARRIER, HALF-LIFE, HEAVY ION FUSION REACTIONS, INTEGRAL CROSS SECTIONS, IRON 58 REACTIONS, LEAD 207 TARGET, LEAD 208 TARGET, MASS DEFECT, MEV RANGE 10-100, MICROSEC LIVING RADIOISOTOPES, MILLISEC LIVING RADIOISOTOPES, NEUTRONS, NUCLEAR STRUCTURE, PROGRESS REPORT, QUASI-FISSION, Q-VALUE, REVIEWS, SHELL MODELS, SPONTANEOUS FISSION, SPONTANEOUS FISSION RADIOISOTO, TITANIUM 50 REACTIONS
ALPHA DECAY RADIOISOTOPES, BARYONS, CROSS SECTIONS, DECAY, DOCUMENT TYPES, ELEMENT 104 ISOTOPES, ELEMENT 105 ISOTOPES, ELEMENT 106 ISOTOPES, ELEMENT 107 ISOTOPES, ELEMENT 108 ISOTOPES, ELEMENT 109 ISOTOPES, ELEMENTARY PARTICLES, ENERGY, ENERGY RANGE, EVEN-EVEN NUCLEI, EVEN-ODD NUCLEI, FERMIONS, FISSION, HADRONS, HEAVY ION REACTIONS, ISOTOPES, MATHEMATICAL MODELS, MEV RANGE, NUCLEAR DECAY, NUCLEAR MODELS, NUCLEAR REACTIONS, NUCLEI, NUCLEONS, NUCLEOSYNTHESIS, ODD-EVEN NUCLEI, ODD-ODD NUCLEI, POTENTIAL ENERGY, RADIOISOTOPES, SECONDS LIVING RADIOISOTOPES, SYNTHESIS, TARGETS
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