Danzl, J. G.
University of Innsbruck (Austria)2010
University of Innsbruck (Austria)2010
AbstractAbstract
[en] Control over all internal and external degrees of freedom of molecules at the level of single quantum states will enable a series of fundamental studies in physics and chemistry. In particular, samples of ground-state molecules at ultralow temperatures and high number densities will allow novel quantum gas studies and future applications in quantum information science. This thesis describes a series of experiments that lead to the production of ultracold and dense samples of alkali dimer molecules in deeply-bound vibrational levels of the singlet electronic ground state and in a single hyperfine sublevel of the rovibronic ground state. Each ground-state molecule is individually trapped in the motional ground state of an optical lattice well. Starting from an atomic Mott-insulator state with optimized double-site occupancy, weakly-bound dimer molecules are efficiently formed on a Feshbach resonance and subsequently transferred to the rovibronic ground state by a stimulated 4-photon process with the Stimulated Raman Adiabatic Passage (STIRAP) technique with >50% efciency. The molecules are trapped in the lattice and have a lifetime of 8 s. Our results present an important step towards Bose-Einstein condensation of ground-state molecules and, when suitably generalized to polar heteronuclear molecules, the realization of dipolar quantum-gas phases in optical lattices. (author)
[de]
Die Kontrolle ueber alle inneren und aeußeren Freiheitsgrade von Molekuelen auf der Ebene von einzelnen Quantenzustaenden wird eine Reihe von grundlegenden Untersuchungen in Physik und Chemie ermoeglichen. Molekuelensembles, die ultratiefe Temperaturen und hohe Teilchendichten vereinigen, werden neuartige Quantengasuntersuchungen und zukuenftige Anwendungen in der Quanteninformation erlauben. Diese Dissertation beschreibt eine Reihe von Experimenten zur Produktion von ultrakalten und dichten Ensembles von Alkali-Dimer Molekuelen in tief gebundenen Vibrationsniveaus des Singulett elektronischen Grundzustandes und in einem definierten Hyperfeinniveau des Rotations-Schwingungs-Grundzustandes. Jedes Grundzustandsmolekuel ist an einem individuellen Gitterplatz eines optischen Gitters im Bewegungsgrundzustand gefangen. Ausgehend von einem atomaren Mott-Isolator-Zustand mit optimierter Anzahl doppelt besetzter Gitterplaetze werden zunaechst schwach gebundene Molekuele an einer Feshbach-Resonanz assoziiert. Diese werden anschließend mit einem stimulierten 4-Photonen uebergang mit Hilfe der Stimulated-Raman-Adiabatic-Passage (STIRAP) Technik in den Rotations-Schwingungs-Grundzustand mit >50 % Effizienz transferiert. Die Grundzustandsmolekuele sind im optischen Gitter gefangen und ihre Lebensdauer betraegt 8 s. Unsere Ergebnisse stellen einen wichtigen Schritt zur Bose-Einstein-Kondensation von Grundzustandsmolekuelen und, wenn sie entsprechend auf polare heteronukleare Molekuele erweitert werden, zur Realisierung von dipolaren Quantengas-Phasen in optischen Gittern dar. (author)Primary Subject
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2010; 191 p; Available from Library of the University of Innsbruck, Innrain 50, 6020 Innsbruck (AT); Thesis (Ph.D.)
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[en] We report on the control of interaction-induced dephasing of Bloch oscillations for an atomic Bose-Einstein condensate in an optical lattice. We quantify the dephasing in terms of the width of the quasimomentum distribution and measure its dependence on time for different interaction strengths which we control by means of a Feshbach resonance. For minimal interaction, the dephasing time is increased from a few to more than 20 thousand Bloch oscillation periods, allowing us to realize a BEC-based atom interferometer in the noninteracting limit
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(c) 2008 The American Physical Society; Country of input: International Atomic Energy Agency (IAEA)
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[en] We perform precision measurements on a Mott-insulator quantum state of ultracold atoms with tunable interactions. We probe the dependence of the superfluid-to-Mott-insulator transition on the interaction strength and explore the limits of the standard Bose-Hubbard model description. By tuning the on-site interaction energies to values comparable to the interband separation, we are able to quantitatively measure number-dependent shifts in the excitation spectrum caused by effective multibody interactions.
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(c) 2011 American Institute of Physics; Country of input: International Atomic Energy Agency (IAEA)
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Vexiau, R.; Bouloufa, N.; Aymar, M.; Danzl, J. G.; Mark, M. J.; Nägerl, H. C.; Dulieu, O., E-mail: olivier.dulieu@lac.u-psud.fr2011
AbstractAbstract
[en] The present paper aims at finding optimal parameters for trapping of Cs2 molecules in optical lattices, with the perspective of creating a quantum degenerate gas of ground-state molecules. We have calculated dynamic polarizabilities of Cs2 molecules subject to an oscillating electric field, using accurate potential curves and electronic transition dipole moments. We show that for some particular wavelengths of the optical lattice, called “magic wavelengths”, the polarizability of the ground-state molecules is equal to the one of a Feshbach molecule. As the creation of the sample of ground-state molecules relies on an adiabatic population transfer from weakly-bound molecules created on a Feshbach resonance, such a coincidence ensures that both the initial and final states are favorably trapped by the lattice light, allowing optimized transfer in agreement with the experimental observation.
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Copyright (c) 2011 EDP Sciences, SIF, Springer-Verlag Berlin Heidelberg; Country of input: International Atomic Energy Agency (IAEA)
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European Physical Journal. D, Atomic, Molecular and Optical Physics; ISSN 1434-6060; ; v. 65(1-2); p. 243-250
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[en] Three interacting particles form a system which is well known for its complex physical behavior. A landmark theoretical result in few-body quantum physics is Efimov's prediction of a universal set of weakly bound trimer states appearing for three identical bosons with a resonant two-body interaction. Surprisingly, these states even exist in the absence of a corresponding two-body bound state and their precise nature is largely independent of the particular type of the two-body interaction potential. Efimov's scenario has attracted great interest in many areas of physics; an experimental test however has not been achieved. We report the observation of an Efimov resonance in an ultracold thermal gas of cesium atoms. The resonance occurs in the range of large negative two-body scattering lengths and arises from the coupling of three free atoms to an Efimov trimer. We observe its signature as a giant three-body recombination loss when the strength of the two-body interaction is varied near a Feshbach resonance. This resonance develops into a continuum resonance at non-zero collision energies, and we observe a shift of the resonance position as a function of temperature. We also report on a minimum in the recombination loss for positive scattering lengths, indicating destructive interference of decay pathways. Our results confirm central theoretical predictions of Efimov physics and represent a starting point from which to explore the universal properties of resonantly interacting few-body systems
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ICAP 2006: 20. international conference on atomic physics; Innsbruck (Austria); 16-21 Jul 2006; (c) 2006 American Institute of Physics; Country of input: International Atomic Energy Agency (IAEA)
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[en] We investigate local three-body correlations for bosonic particles in three dimensions and one dimension as a function of the interaction strength. The three-body correlation function g(3) is determined by measuring the three-body recombination rate in an ultracold gas of Cs atoms. In three dimensions, we measure the dependence of g(3) on the gas parameter in a BEC, finding good agreement with the theoretical prediction accounting for beyond-mean-field effects. In one dimension, we observe a reduction of g(3) by several orders of magnitude upon increasing interactions from the weakly interacting BEC to the strongly interacting Tonks-Girardeau regime, in good agreement with predictions from the Lieb-Liniger model for all strengths of interaction.
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(c) 2011 American Institute of Physics; Country of input: International Atomic Energy Agency (IAEA)
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[en] We explore the rich internal structure of Cs2 Feshbach molecules. Pure ultracold molecular samples are prepared in a CO2-laser trap, and a multitude of weakly bound states is populated by elaborate magnetic-field ramping techniques. Our methods use different Feshbach resonances as input ports and various internal level crossings for controlled state transfer. We populate higher partial-wave states of up to eight units of rotational angular momentum (l-wave states). We investigate the molecular structure by measurements of the magnetic moments for various states. Avoided level crossings between different molecular states are characterized through the changes in magnetic moment and by a Landau-Zener tunneling method. Based on microwave spectroscopy, we present a precise measurement of the magnetic-field-dependent binding energy of the weakly bound s-wave state that is responsible for the large background scattering length of Cs. This state is of particular interest because of its quantum-halo character
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(c) 2007 The American Physical Society; Country of input: International Atomic Energy Agency (IAEA)
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ANGULAR MOMENTUM, BINDING ENERGY, BOUND STATE, CARBON DIOXIDE LASERS, CESIUM, MAGNETIC FIELDS, MAGNETIC MOMENTS, MICROWAVE RADIATION, MICROWAVE SPECTRA, MOLECULAR STRUCTURE, MOLECULES, POTENTIAL ENERGY, S WAVES, SCATTERING LENGTHS, SEISMIC SURFACE WAVES, SPECTROSCOPY, TEMPERATURE RANGE 0000-0013 K, TRAPPING, TRAPS, TUNNEL EFFECT
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[en] We present experimentally derived potential curves and spin-orbit interaction functions for the strongly perturbed A 1Σu+ and b 3Πu states of the cesium dimer. The results are based on data from several sources. Laser-induced fluorescence Fourier transform spectroscopy (LIF FTS) was used some time ago in the Laboratoire Aime Cotton primarily to study the X 1Σg+ state. More recent work at Tsinghua University provides information from moderate resolution spectroscopy on the lowest levels of the b 3Π0u± state as well as additional high-resolution data. From Innsbruck University, we have precision data obtained with cold Cs2 molecules. Recent data from Temple University was obtained using the optical-optical double resonance polarization spectroscopy technique, and finally, a group at the University of Latvia has added additional LIF FTS data. In the Hamiltonian matrix, we have used analytic potentials (the expanded Morse oscillator form) with both finite-difference (FD) coupled-channel and discrete variable representation (DVR) calculations of the term values. Fitted diagonal and off-diagonal spin-orbit functions are obtained and compared with ab initio results from Temple and Moscow State universities.
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(c) 2011 American Institute of Physics; Country of input: International Atomic Energy Agency (IAEA)
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